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Hemma Mistry, Dr. Farzad Behafarid, Dr. Simon R. Bare and Prof. B. Roldan Cuenya Pressure-Dependent Effect of Hydrogen Adsorption on Structural and Electronic Properties of Pt/γ-Al2O3 Nanoparticles ChemCatChem 6

Version of Record online: 15 NOV 2013 | DOI: 10.1002/cctc.201300783

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Catalysts getting in and out of shape: In situ X-ray absorption fine structure spectroscopy reveals a striking 2 D to a 3 D shape transformation in size- and shape-controlled Pt/γ-Al2O3 nanoparticles under increasing H2 pressure at room temperature. In addition, the ability of these particles to adsorb up to 2.5 hydrogen atoms per platinum atom is demonstrated.

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