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Yin Liang, Zhikao Li, Mohamed Nourdine, Salman Shahid and Prof. Kazuhiro Takanabe Methane Coupling Reaction in an Oxy-Steam Stream through an OH Radical Pathway by using Supported Alkali Metal Catalysts ChemCatChem 6

Article first published online: 24 MAR 2014 | DOI: 10.1002/cctc.201400018

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Make it methane: A universal reaction mechanism involved in the oxidative coupling of methane is demonstrated under oxy-stream conditions by using alkali-metal-based catalysts. Rigorous kinetic measurements indicated a reaction mechanism that is consistent with OH radical formation from an H2O–O2 reaction, followed by C[BOND]H activation in CH4 with an OH radical.

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