Stefanie Tschierlei, Martin Presselt, Christian Kuhnt, Arkady Yartsev, Torbjörn Pascher, Villy Sundström, Michael Karnahl, Matthias Schwalbe , Bernhard Schäfer, Sven Rau , Michael Schmitt, Benjamin Dietzek and Jürgen Popp Photophysics of an Intramolecular Hydrogen-Evolving Ru–Pd Photocatalyst Chemistry - A European Journal 15
Article first published online: 25 JUN 2009 | DOI: 10.1002/chem.200900457
Electron transfer on the clock: Photoinduced electron transfer in the hydrogen-evolving photocatalyst [(tbbpy)2Ru(tpphz)PdCl2]2+ is found to take place on a sub-nanosecond timescale. Femtosecond time-resolved spectroscopy highlights the vectorial nature of electron transfer from the photoactive Ru center across the tpphz bridge to the catalytically active Pd center (see picture).
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