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Tao Wang and Prof. Dr. Junliang Zhang Chemoselective C[BOND]C Bond Cleavage of Epoxide Motifs: Gold(I)-Catalyzed Diastereoselective [4+3] Cycloadditions of 1-(1-Alkynyl)oxiranyl Ketones and Nitrones Chemistry - A European Journal 17

Version of Record online: 1 DEC 2010 | DOI: 10.1002/chem.201002395

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Cutting carbon! A novel facile strategy for the C[BOND]C bond cleavage of oxiranyl ketones has been developed. Carbophilic gold(I) activation of the alkyne side chain mediates a heterocyclization and subsequent C[BOND]C bond cleavage (see scheme).

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