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A. Daniel Schofield, Dr. Ainara Nova, Dr. Jonathan D. Selby, Dr. Andrew D. Schwarz, Dr. Eric Clot and Prof. Dr. Philip Mountford Reaction Site Diversity in the Reactions of Titanium Hydrazides with Organic Nitriles, Isonitriles and Isocyanates: Ti[DOUBLE BOND]Nα Cycloaddition, Ti[DOUBLE BOND]Nα Insertion and Nα[BOND]Nβ Bond Cleavage Chemistry - A European Journal 17

Version of Record online: 15 DEC 2010 | DOI: 10.1002/chem.201002776

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Ti-hydrazide transformations: A range of transformations of the Ti[DOUBLE BOND]NNPh2 functional group with unsaturated organic substrates leading to Ti[DOUBLE BOND]Nα [2+2] cycloaddition, Ti[DOUBLE BOND]Nα insertion or Nα[BOND]Nβ bond cleavage products (see scheme) is reported. A DFT study of the mechanisms of the last two reaction types is described.

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