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Anastasia A. Grishina, Dr. Svetlana M. Polyakova, Roman A. Kunetskiy, Dr. Ivana Císařová and Dr. Ilya M. Lyapkalo 4,5-Disubstituted N,N′-Di-tert-alkyl Imidazolium Salts: New Synthesis and Structural Features Chemistry - A European Journal 17

Article first published online: 7 DEC 2010 | DOI: 10.1002/chem.201002805

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It's getting crowded! The synthesis of a new subfamily of imidazolium cations with exceptionally spatially demanding substitution patterns (see scheme) paved the way to reconcile two antagonising effects: steric hindrance and innately high donating ability/basicity in the peralkylated imidazol-2-ylidene ligands/uncharged bases.

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