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Dr. Sven Tobisch Does a Concerted Non-Insertive Mechanism Prevail over a σ-Insertive Mechanism in Catalytic Cyclohydroamination by Magnesium Tris(oxazolinyl)phenylborate Compounds? A Computational Study Chemistry - A European Journal 17

Article first published online: 25 NOV 2011 | DOI: 10.1002/chem.201101490

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Rival mechanistic pathways for C[DOUBLE BOND]C bond activation in alkaline-earth metal-catalysed hydroamination: Computational mechanistic analysis provides sound evidence for the operation of an (ToM)Mg[BOND]N amido σ-bond insertive mechanism with turnover-limiting aminolysis for aminoalkene cyclohydroamination (see scheme).

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