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Ludovic Castro and Prof. Dr. Laurent Maron Insight into the Reaction Mechanisms of (MeC5H4)3U with Isoelectronic Heteroallenes CS2, COS, PhN3, and PhNCO by DFT Studies: A Unique Pathway that Involves Bimetallic Complexes Chemistry - A European Journal 18

Article first published online: 18 APR 2012 | DOI: 10.1002/chem.201103754

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U are always on my mind: The mechanisms for the reactions of four isoelectronic heteroallenes (see figure) with the trivalent uranium complex (MeC5H4)3U were determined by DFT methods. The unique reaction mechanism involved a uranium(IV) bimetallic complex with a bridged heteroallene intermediate.

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