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Christopher M. Kareis, Dr. Jae-Hyuk Her, Prof. Peter W. Stephens, Dr. Joshua G. Moore and Prof. Joel S. Miller Structure and Magnetic Ordering of the Anomalous Layered (2D) Ferrimagnet [NEt4]2MnII3(CN)8 and 3D Bridged-Layered Antiferromagnet [NEt4]MnII3(CN)7 Prussian Blue Analogues Chemistry - A European Journal 18

Version of Record online: 19 JUN 2012 | DOI: 10.1002/chem.201200672

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Prussian virtues: The reaction of [NEt4]CN and Mn(O2CMe)2 unexpectedly formed [NEt4]MnII3(CN)7 and [NEt4]2MnII3(CN)8 solvated materials; these are distinctly different to previously characterized members of the Prussian blue family. These unexpected stoichiometries, layered and bridged-layered structures (see figure), as well as their magnetic ordering, are reported herein.

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