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Xiang-Wei Liu, Yan Yan, Yong-Qiang Wang, Chao Wang and Prof. Dr. Jian Sun Highly Enantioselective Reduction of β-Amino Nitroolefins with a Simple N-Sulfinyl Urea as Bifunctional Catalyst Chemistry - A European Journal 18

Version of Record online: 26 JUN 2012 | DOI: 10.1002/chem.201201192

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Simple but effective: A structurally simple N-sulfinyl urea was found to be a highly efficient bifunctional catalyst, which allows for the development of a novel pathway for the construction of chiral β-amino nitroalkanes through enantioselective reduction of β-amino nitroolefins by trichlorosilane. High yields and excellent enantioselectivities were obtained for a broad range of β-arylamino nitroolefin substrates (see scheme).

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