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Toshiki Nagamachi, Dr. Youhei Takeda, Kazuhisa Nakayama and Prof. Dr. Satoshi Minakata Selective Functionalization of Fullerenes with N,N-Dihalosulfonamides as an N1 Unit: Versatile Syntheses of Aza[60]fulleroids and Aziridino[60]fullerenes and their Application to Photovoltaic Cells Chemistry - A European Journal 18

Article first published online: 14 AUG 2012 | DOI: 10.1002/chem.201201680

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Full steam ahead: Highly selective and versatile syntheses of aza[60]fulleroids and aziridino[60]fullerenes from C60, which utilize N,N-dihalosulfonamides as an N1 source, were developed. Photophysical, electrochemical, and thermal properties of the iminofullerenes were measured, and photovoltaic cells based on these compounds were fabricated. The power conversion efficiencies (PCEs) of the devices show moderate values ranging from 1.33 to 2.35 % (see scheme).

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