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Dr. Matthias Vogt, Moti Gargir, Dr. Mark A. Iron, Dr. Yael Diskin-Posner, Yehoshoa Ben-David and Prof. Dr. David Milstein A New Mode of Activation of CO2 by Metal–Ligand Cooperation with Reversible C[BOND]C and M[BOND]O Bond Formation at Ambient Temperature Chemistry - A European Journal 18

Article first published online: 26 JUN 2012 | DOI: 10.1002/chem.201201730

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Team work: Although CO2 binding to metal centers usually involves π coordination to a C[DOUBLE BOND]O group or σ bonds to the carbon or oxygen atom of the CO2 molecule, a new mode of metal–ligand cooperative activation of CO2 to a ruthenium PNP pincer complex involving aromatization/dearomatization steps is presented in experimental and theoretical studies (see scheme).

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