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Yong-Jun Bian, Chao-Yue Chen and Prof. Zhi-Zhen Huang  Synthesis of Imides by Palladium-Catalyzed C[BOND]H Functionalization of Aldehydes with Secondary Amides Chemistry - A European Journal 19

Version of Record online: 13 NOV 2012 | DOI: 10.1002/chem.201202601

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An efficient palladium-catalyzed C[BOND]H functionalization of aldehydes with various N-substituted N-heteroarene-2-carboxamides has been developed for the synthesis of secondary imides (see scheme; TBHP=tert-butyl hydroperoxide). The reaction tolerates various functional groups. A tentative radical mechanism for a PdII/PdIV catalytic cycle is proposed.

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