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Zhongyue Zhang, Dr. Hanhua Zhao, Hirotaka Kojima, Prof. Takehiko Mori and Prof. Kim R. Dunbar Conducting Organic Frameworks Based on a Main-Group Metal and Organocyanide Radicals Chemistry - A European Journal 19

Version of Record online: 23 JAN 2013 | DOI: 10.1002/chem.201203422

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Main-group semiconductors: New 2,5-dihalogen-substituted [Tl(TCNQX2)] (TCNQ=7,7,8,8-tetracyanoquinodimethane, X=H, Cl, Br, I) derivatives reveal potential for the realization of unprecedented molecule-based main-group semiconductors (see figure). The theoretical simulation of band structures hints at modulation of the 1D band structure by the TlI cations.

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