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Melissa J. MacDonald, Colin R. Hesp, Derek J. Schipper, Marc Pesant and Prof. André M. Beauchemin Highly Enantioselective Intermolecular Hydroamination of Allylic Amines with Chiral Aldehydes as Tethering Catalysts Chemistry - A European Journal 19

Version of Record online: 10 JAN 2013 | DOI: 10.1002/chem.201203462

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Chirally LinkedIn: Chiral aldehydes are effective tethering catalysts for enantioselective intermolecular hydroamination, which provides access to vicinal diamine motifs in good yields and excellent enantioselectivities (see scheme). This work highlights simple chiral α-oxygenated aldehydes as effective organocatalysts capable of efficiently inducing asymmetry through transient intramolecularity.

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