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Lei Ren, Xiao-Lei Lian and Prof. Liu-Zhu Gong Brønsted Acid/Rhodium(II) Cooperative Catalytic Asymmetric Three-Component Aldol-Type Reaction for the Synthesis of 3-Amino Oxindoles Chemistry - A European Journal 19

Article first published online: 10 FEB 2013 | DOI: 10.1002/chem.201203993

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Cooperation is key! Chiral Brønsted acid/rhodium(II) cooperative catalysis enabled an enantioselective three-component aldol-type reaction of 3-diazo oxindoles and anilines with glyoxylates to give highly functionalized and structurally diverse 3-amino oxindoles in high stereoselectivity (>20:1 d.r., 99 % ee; see scheme).

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