Dr. Christian Perbandt, Vanessa Bacher, Michael Groves, Dr. Meinhard Schwefer, Dr. Rolf Siefert and Prof. Dr.-Ing. Thomas Turek Kinetics and Reactor Design for N2O Decomposition in the EnviNOx® Process Chemie Ingenieur Technik 85
The reaction kinetics of N2O decomposition on a commercial iron zeolite catalyst was determined by systematic measurements for typical conditions in nitric acid plant tail gases. Based on these measurements, a reactor model was developed that takes into account mass transfer resistances, axial dispersion and pressure drop. With this model, different options for the catalyst geometry were compared quantitatively.
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