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Arthur R. G. Smith, Prof. Paul L. Burn and Prof. Ben J. Powell Spin–Orbit Coupling in Phosphorescent Iridium(III) Complexes ChemPhysChem 12

Article first published online: 22 JUL 2011 | DOI: 10.1002/cphc.201100397

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Exciting couples: The excited-state properties of two iridium(III) complexes with potential applications in organic light-emitting diodes are calculated (see picture). An indirect relativistic stabilisation of the metal-to-ligand charge transfer states increases the effectiveness of spin–orbit coupling in hybridising singlet and triplet states, thus enhancing phosphoresce.

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