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Thomas Waldmann, Jens Klein, Prof. Dr. Harry E. Hoster and Prof. Dr. R. Jürgen Behm Stabilization of Large Adsorbates by Rotational Entropy: A Time-Resolved Variable-Temperature STM Study ChemPhysChem 14

Article first published online: 9 OCT 2012 | DOI: 10.1002/cphc.201200531

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Big is best: Bis(terpyridine) adsorbates on a Ag(111) surface in combination with large data sets from scanning tunneling microscopy and statistical mechanics calculations are used as a model system for entropic stabilization of large rotating adsorbates (see picture). The general validity of this concept is tested for other typical small, mid-sized and large adsorbates.

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