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Dr. Gernot Füchsel, Dr. Jean Christophe Tremblay, Dr. Tillmann Klamroth and Prof. Dr. Peter Saalfrank Quantum Dynamical Simulations of the Femtosecond-Laser-Induced Ultrafast Desorption of H2 and D2 from Ru(0001) ChemPhysChem 14

Version of Record online: 20 FEB 2013 | DOI: 10.1002/cphc.201200940

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Las-ing around: Quantum mechanical desorption induced by electronic transition simulations in 3D is reported to describe the recombinative desorption of H2 and D2 from Ru(0001) produced by low-intensity laser fields. The experimental trends at low laser fluences are well reproduced for the isotopic ratio and the translational and rotational energies. A single temperature is sufficient to characterize the energy distributions for all degrees of freedom.

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