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Alberto Castro Theoretical Shaping of Femtosecond Laser Pulses for Ultrafast Molecular Photo-Dissociation with Control Techniques Based on Time-Dependent Density Functional Theory ChemPhysChem 14

Version of Record online: 26 MAR 2013 | DOI: 10.1002/cphc.201201021

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Ultrafast and optimal: optimal ultrashort pulses are theoretically constructed by the combination of time-dependent density functional theory and optimal control, optimizing the classical opposing force on the nuclei for the hydrogen molecule (see picture; top panel: internuclear distance and the bound electrons count; bottom panel: opposing force; gray region: pulse duration).

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