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Dr. Yasuki Arasaki and Prof. Dr. Kazuo Takatsuka Pulse-Train Photoelectron Spectroscopy of Electronic and Nuclear Dynamics in Molecules ChemPhysChem 14

Version of Record online: 29 APR 2013 | DOI: 10.1002/cphc.201201094

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Fast train: A femtosecond pulse train causes step-like electronic population transfers together with photoionization (see picture). The history of the electronic and vibrational excitation is theoretically shown to be reflected in the time evolution of the photoelectron kinetic energy distribution, leading to a novel and direct way for the investigation of dynamics involving multiple excited states.

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