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Peiyu Ge, Astrid J. Olaya, Dr. Micheál D. Scanlon, Dr. Imren Hatay Patir, Heron Vrubel and Prof. Hubert H. Girault Photoinduced Biphasic Hydrogen Evolution: Decamethylosmocene as a Light-Driven Electron Donor ChemPhysChem 14

Version of Record online: 17 MAY 2013 | DOI: 10.1002/cphc.201300122

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A weak but productive donor: Mechanistic and kinetic insights into light-driven biphasic hydrogen evolution in the presence of the weak electron donor decamethylosmocene , which on white-light illumination produces an excited-state species that can reduce organically solubilized protons (see picture), are obtained by gas chromatographic, cyclic voltammetric, and UV/Vis and 1H NMR spectroscopic analysis.

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