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Johann Förster and Dr. Alejandro Saenz Theoretical Study of the Inversion Motion of the Ammonia Cation with Subfemtosecond Resolution for High-Harmonic Spectroscopy ChemPhysChem 14

Article first published online: 12 APR 2013 | DOI: 10.1002/cphc.201300180

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The autocorrelation functions for the umbrella motion of the ammonia cation are calculated explicitly using a one-dimensional model. This explains the occurrence of the previously predicted maximum in the ratio of the autocorrelation functions. Furthermore, different initial states and two different ways of incorporating strong-field corrections to the Franck–Condon approximation are briefly discussed.

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