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Dr. Ross J. Ellis and Dr. Mark R. Antonio Redox Chemistry of Third Phases Formed in the Cerium/Nitric Acid/Malonamide-n-Dodecane Solvent Extraction System ChemPlusChem 77

Article first published online: 30 DEC 2011 | DOI: 10.1002/cplu.201100022

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Three phases are a charm: The electroactive nature of Ce and its renowned CeIII/IV couple make it the keystone of this investigation at the intersection of separation science and electrochemistry. The CeIII/IV couple has been probed to disclose its physical and spectroscopic behaviors in organic phases of relevance to solvent extraction, thus affording original insights into third phase phenomena and ion transfer across the aqueous–organic liquid interface in the title system (see figure).

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