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Kolleboyina Jayaramulu, Dr. Kasibhatta K. R. Datta, Mothika V. Suresh, Gayatri Kumari, Dr. Ranjan Datta, Prof. Chandrabhas Narayana, Prof. Muthusamy Eswaramoorthy and Prof. Tapas Kumar Maji Honeycomb Porous Framework of Zinc(II): Effective Host for Palladium Nanoparticles for Efficient Three-Component (A3) Coupling and Selective Gas Storage ChemPlusChem 77

Version of Record online: 21 JUN 2012 | DOI: 10.1002/cplu.201200093

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MOF for effective stabilizer for “Pd” and selective host for CO2: A porous, layered MOF system {[Zn(Himdc)(bipy)].DMF} (1; Himdc=4,5-imidazoledicarboxylate, bipy=4,4'-bipyridine) shows selective gas-storage properties, while the polar nanochannels serve as functional scaffold for the stabilization of highly dispersed Pd nanoparticles. The Pd@MOF1 a hybrid is a highly active and recyclable catalyst for the synthesis of propargylamine derivatives through A3 coupling reactions.

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