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Oliver Krahe, Prof. Dr. Frank Neese and Dr. Marianne Engeser Iron Azides with Cyclam-Derived Ligands: Are They Precursors for High-Valent Iron Nitrides in the Gas Phase? ChemPlusChem 78

Version of Record online: 5 JUL 2013 | DOI: 10.1002/cplu.201300182

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High-valent iron nitrides: Azide complexes as their potential precursors are studied in the gas phase by mass spectrometry. A subtle interplay between pathways to FeII, FeIII, and FeV products is controlled by choice of the ligand (see figure). The observations partly parallel those seen after irradiating frozen solutions.

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