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Dr. Miklos Czaun, Dr. Alain Goeppert, Robert May, Dr. Ralf Haiges, Prof. Dr. G. K. Surya Prakash and Prof. Dr. George A. Olah Hydrogen Generation from Formic Acid Decomposition by Ruthenium Carbonyl Complexes. Tetraruthenium Dodecacarbonyl Tetrahydride as an Active Intermediate ChemSusChem 4

Version of Record online: 14 MAR 2011 | DOI: 10.1002/cssc.201000446

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Renewable energy carrier: Carbonylation and hydrido carbonylation of ruthenium halides by formic acid is reviewed. The first preparation of [Ru4(CO)12H4], using formic acid as the exclusive CO and hydride source, and the catalytic activity of [Ru4(CO)12H4] for the decomposition of formic acid to CO2 and H2 are also reported.

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