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Dr. Kambiz Chizari, Dr. Adrien Deneuve, Dr. Ovidiu Ersen, Dr. Ileana Florea, Dr. Yu Liu, Prof. David Edouard, Dr. Izabela Janowska, Dr. Dominique Begin and Dr. Cuong Pham-Huu Nitrogen-Doped Carbon Nanotubes as a Highly Active Metal-Free Catalyst for Selective Oxidation ChemSusChem 5

Version of Record online: 1 DEC 2011 | DOI: 10.1002/cssc.201100276

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Nanotubes say goodbye to H2S: Nitrogen-doped carbon nanotubes (N-CNTs) are synthesized by using a chemical vapor deposition method under a mixture of C2H6/NH3/Ar with Fe/Al2O3 as a growth catalyst. N-CNTs can be used as a metal-free catalyst for the selective oxidation of H2S into elemental sulfur. The desulfurization activity can be further improved by supporting the N-CNT on a macroscopic host structure such as SiC foam.

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