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Xueqiang Li, Prof. Mei Wang, Lin Chen, Xiuna Wang, Jingfeng Dong and Prof. Licheng Sun Photocatalytic Water Reduction and Study of the Formation of FeIFe0 Species in Diiron Catalyst Sytems ChemSusChem 5

Article first published online: 8 MAR 2012 | DOI: 10.1002/cssc.201100490

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Three gang up on hydrogen: Bioinspired diiron complexes, xanthene dyes, and triethylamine make up three-component systems that display high turnover numbers for the photoinduced hydrogen production. The quantum yield is determined for this catalytic system. A plausible mechanism for the formation of the FeIFe0 species is proposed, which involves the reduction of the diiron catalyst by the neutral alkyl radical photogenerated from triethylamine.

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