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Siddulu N. Talapaneni, Gurudas P. Mane, Ajayan Mano, Dr. Chokkalingam Anand, Dr. Dattatray S. Dhawale, Prof. Toshiyuki Mori and Prof. Ajayan Vinu Synthesis of Nitrogen-Rich Mesoporous Carbon Nitride with Tunable Pores, Band Gaps and Nitrogen Content from a Single Aminoguanidine Precursor ChemSusChem 5

Version of Record online: 2 MAR 2012 | DOI: 10.1002/cssc.201100626

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Tune in, see the pores: We report on the synthesis of N-rich mesoporous carbon nitrides (CNs) with tunable pore diameters, N content, and band gaps through hard templating using a single aminoguanidine molecule as a CN precursor, which shows a much higher activity for Friedel–Crafts acylation of benzene with hexanoyl chloride as compared to other CNs with and without a mesoporous structure. We expect that these materials may be used in photoelectrochemical applications.

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