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Dr. Angela Kruth, Sven Hansen, Dr. Torsten Beweries, Dr. Volker Brüser and Prof. Dr. Klaus-Dieter Weltmann Plasma Synthesis of Polymer-Capped Dye-Sensitised Anatase Nanopowders for Visible-Light-Driven Hydrogen Evolution ChemSusChem 6

Version of Record online: 26 NOV 2012 | DOI: 10.1002/cssc.201200408

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To sensitise and encapsulate: Ru dye-sensitised TiO2 is encapsulated with plasma-polymerised polyallylamine to improve long-term stability under ambient conditions for photocatalytic water splitting. Using a Pd dichloro complex as the reduction catalyst and triethylamine as the electron source, a highly stable long-term performance as well as a small improvement in catalytic activity is achieved. The nanostructure is characterised by TEM as well as UV/Vis and ATR-FTIR spectroscopy.

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