Christof Aellig, David Scholz and Prof. Dr. Ive Hermans Metal-Free Aerobic Alcohol Oxidation: Intensification under Three-Phase Flow Conditions ChemSusChem 5
The aerobic oxidation of primary and secondary alcohols under the influence of a solid acid catalyst is presented. Process optimization and intensification through the use of a continuous three-phase flow reactor is demonstrated. Space–time yields are found to increase by two orders of magnitude with respect to batch experiments, along with additional gains in selectivity and a decrease of N2O formation.
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