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Jingfeng Dong, Prof. Mei Wang, Xueqiang Li, Lin Chen, Yu He and Prof. Licheng Sun Simple Nickel-Based Catalyst Systems Combined With Graphitic Carbon Nitride for Stable Photocatalytic Hydrogen Production in Water ChemSusChem 5

Article first published online: 30 OCT 2012 | DOI: 10.1002/cssc.201200490

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A molecular catalyst system containing only earth-abundant elements is combined with g-C3N4 as photosensitizer. The in situ generated complexes serve as catalysts for visible-light-driven H2 production in aqueous solution, and do not require organic solvent or a Brønsted acid. H2 evolution from the Ni-based catalyst system can be maintained for over 60 h, demonstrating that the combination is a promising approach to improve the lifetimes of molecular catalysts towards photochemical H2 production.

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