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Hui Ren, Weiting Yu, Michael Salciccioli, Ying Chen, Yulin Huang, Ke Xiong, Prof. Dionisios G. Vlachos and Prof. Jingguang G. Chen Selective Hydrodeoxygenation of Biomass-Derived Oxygenates to Unsaturated Hydrocarbons using Molybdenum Carbide Catalysts ChemSusChem 6

Version of Record online: 4 APR 2013 | DOI: 10.1002/cssc.201200991

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Which cleavage do you prefer? With a combination of density functional theory (DFT) calculations, surface science studies, and reactor evaluations, Mo2C is identified as a highly selective HDO catalyst to selectively convert biomass-derived oxygenates to unsaturated hydrocarbons through selective C[BOND]O bond scissions without C[BOND]C bond cleavage. This provides high-value HDO products for utilization as feedstocks for chemicals and fuels; this also reduces the overall consumption of H2.

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