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Peter Sponholz, Dörthe Mellmann, Dr. Henrik Junge and Prof. Matthias Beller Towards a Practical Setup for Hydrogen Production from Formic Acid ChemSusChem 6

Article first published online: 11 JUN 2013 | DOI: 10.1002/cssc.201300186

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Formic acid cracker: A mini plant that allows for continuous formic acid decomposition to hydrogen and carbon dioxide under ambient conditions is presented. By using an in situ-formed ruthenium catalyst, unprecedented turnover numbers over 1 000 000 are achieved. The active catalyst is formed in situ from commercially available [RuCl2(benzene)]2 and 1,2-bisdiphenylphosphinoethane.

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