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Prof. Guisheng Li, Peng Zhang, Prof. Zhenfeng Bian, Prof. Jian Zhu, Ling Wu and Prof. Hexing Li Mesoporous TiN Microspheres with Hierarchical Chambers and Enhanced Visible Light-Driven Hydrogen Evolution ChemSusChem 6

Article first published online: 19 JUN 2013 | DOI: 10.1002/cssc.201300221

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Open into the light: Mesoporous titanium nitride (TiN) microspheres with tunable structures are synthesized through NH3 nitridation and structure duplication of organotitania. The yolk–shell TiN demonstrates high H2 yield in visible light-induced photocatalytic water splitting owing to a narrow energy band gap, unique chamber structure, high surface area, and excellent electrical conductivity, which promoted light harvesting, reactant adsorption, and photoelectron–hole separation.

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