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Dr. Liling Fu, Dr. Genggeng Qi, Dr. Osama Shekhah, Dr. Youssef Belmabkhout, Dr. Luis Estevez, Prof. Mohamed Eddaoudi and Prof. Emmanuel P. Giannelis Synthesis and Carbon Dioxide Sorption of Layered Double Hydroxide/Silica Foam Nanocomposites with Hierarchical Mesostructure ChemSusChem 7

Article first published online: 5 MAR 2014 | DOI: 10.1002/cssc.201300973

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Respect the hierarchy: Hierarchical mesoporous layered double hydroxide (LDH) nanocomposites with high surface areas and large pore volumes are synthesized by controlled hydrothermal growth of LDH precursors on a mesoporous silica foam. The as-synthesized nanocomposites exhibit a significantly enhanced capacity and selectivity towards carbon dioxide, making them very promising candidates for carbon dioxide (CO2) separation applications.

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