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Nicholas D. McNamara and Prof. Jason C. Hicks CO2 Capture and Conversion with a Multifunctional Polyethyleneimine-Tethered Iminophosphine Iridium Catalyst/Adsorbent ChemSusChem 7

Version of Record online: 3 MAR 2014 | DOI: 10.1002/cssc.201301231

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Balancing act: A tunable, multifunctional, solid material able to both capture CO2 and subsequently convert it to formic acid is synthesized by the modification of polyethyleneimine with an iminophosphine ligand and an Ir precatalyst. By altering the structure of the material, a balance between capture and conversion is reached, which results in an optimal multifunctional material.

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