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Dr. Athanassios G. Kontos, Dr. Vlassis Likodimos, Dr. Charitomeni M. Veziri, Dr. Evangelos Kouvelos, Nikolaos Moustakas, Dr. Georgios N. Karanikolos, Dr. George Em. Romanos and Dr. Polycarpos Falaras CO2 Captured in Zeolitic Imidazolate Frameworks: Raman Spectroscopic Analysis of Uptake and Host–Guest Interactions ChemSusChem 7

Article first published online: 28 MAR 2014 | DOI: 10.1002/cssc.201301323

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Are you Raman enough? In situ Raman investigation of the interactions of zeolitic imidazolate frameworks (ZIFs) with CO2 in practical pressure and temperature regimes (0–10 bar and 0–64 °C) correlates well with corresponding macroscopic CO2 sorption data and shows clear spectroscopic evidence of CO2 uptake (see image). Raman is found to be an easy and sensitive tool for quantifying CO2 uptake, identifying weak host–guest interactions, and elucidating CO2 sorption mechanism in ZIFs.

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