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Danim Yun, Tae Yong Kim, Dae Sung Park, Yang Sik Yun, Prof. Jeong Woo Han and Prof. Jongheop Yi A Tailored Catalyst for the Sustainable Conversion of Glycerol to Acrolein: Mechanistic Aspect of Sequential Dehydration ChemSusChem 7

Version of Record online: 8 JUL 2014 | DOI: 10.1002/cssc.201402057

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A maze of holes and acid is all it takes: A highly stable and selective catalyst for the sequential dehydration of glycerol to acrolein is presented. Outstanding performance is achieved due to the superior recyclability of Brønsted acid sites and hierarchical structure with meso- and macropores. The former hinders 3-hydroxypropionaldehyde degradation during sequential dehydration and the latter enhances the intrinsic coke resistivity.

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