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Daniel L. DuBois and R. Morris Bullock Molecular Electrocatalysts for the Oxidation of Hydrogen and the Production of Hydrogen – The Role of Pendant Amines as Proton Relays European Journal of Inorganic Chemistry 2011

Version of Record online: 4 JAN 2011 | DOI: 10.1002/ejic.201001081

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Pendant amines function as proton relays in molecular electrocatalysts, facilitating transfer of protons to and from the metal. A series of NiII complexes with diphosphanes bearing pendant amines are catalysts for oxidation of H2, and a related series of NiII and CoII complexes catalyze the production of H2 by reduction of protons.

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