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Alexios Grigoropoulos, Dimitrios Maganas, Dimitrios Symeonidis, Petros Giastas, Andrew R. Cowley, Panayotis Kyritsis and Georgios Pneumatikakis Synthesis of Chalcogenidoimidodiphosphinato–RhI Complexes and DFT Investigation of Their Catalytic Activation in Olefin Hydroformylation European Journal of Inorganic Chemistry 2013

Version of Record online: 19 DEC 2012 | DOI: 10.1002/ejic.201200921

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The different catalytic properties of mono- and dichalcogenidoimidodiphosphinato–RhI complexes have been investigated through a combined experimental and computational approach. The results indicate that catalytic activation proceeds by means of the ligand-assisted heterolytic cleavage of H2.

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