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Gavin A. Craig, José Sánchez Costa, Olivier Roubeau, Simon J. Teat and Guillem Aromí An FeII Spin-Crossover Complex Becomes Increasingly Cooperative with Ageing European Journal of Inorganic Chemistry 2013

Version of Record online: 21 NOV 2012 | DOI: 10.1002/ejic.201201041

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Improving with ageing! A bpp-type [bpp = bis(pyrazol-3-yl)pyridine)] ligand, H4L, designed to enhance intermolecular interactions, leads to the spin-crossover (SCO) compound [Fe(H4L)2](ClO4)2·2THF·H2O, which exhibits enhanced spin transition cooperativity with ageing. The intermolecular interactions as a whole are analysed and compared with those of related compounds by the use of Hirshfeld diagrams.

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