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Darunee Sertphon, David J. Harding, Phimphaka Harding, Keith S. Murray, Boujemaa Moubaraki, John D. Cashion and Harry Adams Anionic Tuning of Spin Crossover in FeIII–Quinolylsalicylaldiminate Complexes European Journal of Inorganic Chemistry 2013

Version of Record online: 26 NOV 2012 | DOI: 10.1002/ejic.201201066

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A series of new spin-crossover FeIII complexes, [FeIII(qsal-5-OMe)2]Y [Y = BF4 (1), PF6 (2), NCS (3), BPh4 (4)], are reported. Structural, magnetic and Mössbauer spectroscopic studies have revealed that the size and shape of the anion are crucial for controlling the nature or absence of spin crossover.

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