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Iwona Kuźniarska-Biernacka, Otilia Rodrigues, Maria Alice Carvalho, Pier Parpot, Krzysztof Biernacki, Alexandre Lopes Magalhães, Antonio Mauricio Fonseca and Isabel Correia Neves Electrochemical and Catalytic Studies of a Manganese(III)Complex with a Tetradentate Schiff-Base Ligand Encapsulated in NaY Zeolite European Journal of Inorganic Chemistry 2013

Version of Record online: 4 APR 2013 | DOI: 10.1002/ejic.201201517

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Two methods for the encapsulation of a MnIIIsalen complex in NaY zeolite lead to different modes of coordination at the metal. Cyclic voltammetry of the neat and heterogeneous complexes shows different electrochemical behaviour. The heterogeneous catalysts lead to similar or higher alkene conversion than the homogeneous catalyst. DFT confirmed distortion of the complex in a confined space.

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