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Bin Zhang, Yan Zhang, Zengqiang Gao, Guangcai Chang, Shaokui Su, Dongwei Wang, Yanjun Guo and Daoben Zhu Synthesis, Crystal Structure, and Characterization of the Charge-Transfer Salt (BEDT-TTF)[Fe(C2O4)Cl2](CH2Cl2), {BEDT-TTF = Bis(ethylenedithio)tetrathiafulvalene} European Journal of Inorganic Chemistry 2014

Version of Record online: 20 MAY 2014 | DOI: 10.1002/ejic.201402112

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The title compound has been synthesized and studied, and it was found that the donor layers in the organic–inorganic hybrid charge-transfer salt, which is composed of BEDT-TTF1.0+ dimers and CH2Cl2, are separated by zigzaged anion chains. The compound is a semiconductor and shows strong antiferromagnetic interactions between the oxalate-bridged metal atoms.

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