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Anne Grundmann, Menyhárt B. Sárosi, Peter Lönnecke and Evamarie Hey-Hawkins Organotantalum Phosphaketene and Phosphaazaallene Complexes European Journal of Inorganic Chemistry 2014

Article first published online: 4 JUN 2014 | DOI: 10.1002/ejic.201402400

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The first tantalum phosphaketene and phosphaazaallene complexes are obtained by insertion of carbon monoxide and cyclohexyl isocyanide into the Ta–P bond of cyclohexyl- and (isopropylphosphanylidene)tantalum(V) complexes. The phosphaazaallene complexes occur as E and Z isomers. These isomers have different electronic structures according to NMR spectroscopy studies and DFT calculations.

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