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Giuseppe Lanza, Maria A. Chiacchio, Salvatore V. Giofrè, Roberto Romeo and Pedro Merino The High Selectivity of the Cp2ZrHCl Reducing Agent for Imides: A Combined Experimental and Theoretical Study on γ-Lactam and Isoxazolidinone Derivatives European Journal of Organic Chemistry 2013

Version of Record online: 21 NOV 2012 | DOI: 10.1002/ejoc.201201186

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Semicyclic imides such as γ-lactam and isoxazolidinone derivatives are efficiently and selectivity reduced by the Cp2ZrHCl agent. The energetic reaction pathways for endo and exo attack, computed at the DFT level including thermal effects, allow an exhaustive interpretation of current and previously reported experimental data.

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