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M. Dhyne, M. Lepère and P. Joubert Semiclassical line broadening calculations, using an ab initio potential energy surface, in Q-branch and S-branch of N2 perturbed by H2 Journal of Raman Spectroscopy 43

Article first published online: 16 JUL 2012 | DOI: 10.1002/jrs.4126

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H2 broadening coefficients of Raman lines belonging to Q-branch and S-branch of N2 have been calculated using a numerical procedure based on the semiclassical Robert–Bonamy model. With the ab initio potential energy surface used, results are obtained for a large range of temperatures and J quantum numbers and compared with a satisfactory agreement with previous experimental data.

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